Badtke, MoritzMoritzBadtkePüschel, StefanStefanPüschelLiestmann, ZoeZoeLiestmannTanaka, HirokiHirokiTanakaKränkel, ChristianChristianKränkelKalusniak, SaschaSaschaKalusniak2025-05-062025-05-062025https://publica.fraunhofer.de/handle/publica/48729510.1364/OE.5594282-s2.0-105001360471Tm3+-doped YLF crystals with different doping concentrations are grown and investigated for their suitability for continuous-wave laser operation on the 3H4→3F4 transition around 1.5 µm. Our spectroscopic investigations reveal the emission, absorption, and gain cross sections as well as the concentration-dependent lifetime of the relevant energy levels. Self-termination of the laser is circumvented in a cascade laser scheme 3H4→3F4→3H6 for efficient depopulation of the long-living lower laser level 3F4. In this way, simultaneous laser operation at 1509 nm and 1923 nm with slope efficiencies of 44% and 35% and pump-power-limited output powers of 590 mW and 670 mW are obtained under 781-nm Ti:sapphire laser pumping, respectively.entruejournal article